Her 2011 sophomore record has beaten the likes of Susan Boyle and Mumford & Sons to the title, after scoring the most digital and physical sales on the website over the past three years.
SuBo's debut album, I Dreamed A Dream, is behind Adele in second place, while Stephen Schwartz and the original Broadway cast of Wicked are at No.3.
Taylor Swift, Amy Winehouse and Coldplay also feature in the Top Ten, with Adele's first record 19, is in eighth place.
Lady Gaga's Born This Way has also been named the best-selling MP3 album of all time, after Amazon offered Mother Monster's LP for just 99 cents during its first week on sale in 2011.
Daft Punk's comeback album Random Access Memories was also named the best-selling CD on Amazon in 2013.
Robin Thicke's Blurred Lines was named the best-selling MP3 single of the year, while Katy Perry and Roar were in second place.
Amazon.com's best-selling albums of all time - Top 10:
1. Adele: 21
2. Susan Boyle: I Dreamed A Dream
3. Stephen Schwartz: Wicked (2003 Original Broadway Cast)
4. Robert Plant & Alison Krauss: Raising Sand
5. Mumford & Sons: Sigh No More
6. Taylor Swift: Fearless
7. Amy Winehouse: Back to Black
8. Adele: 19
9. Dixie Chicks: Taking the Long Way
10. Coldplay: Viva la Vida or Death and All His Friends
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